Enhancing the Self-Propelled Motion of Hydrogen Peroxide Fueled Active Particles with Formic Acid and Other Oxygen Scavengers. Journal Article uri icon

Overview

abstract

  • We report enhanced active particle motion in hydrogen peroxide-fueled self-diffusiophoretic active particle systems of up to 400% via addition of low concentrations of oxygen scavenging agents such as formic acid (as well as other organic acids, hydrazine, and citric acid), whereas active motion was inhibited at higher concentrations. Control experiments showed that enhanced motion was decoupled from catalytic hydrogen peroxide decomposition rate and insensitive to particle surface chemistry. Experimental results point to bulk oxygen scavenging as the cause for the enhanced active motion, representing a realization of recently predicted promotional effects of product sinks on self-diffusiophoretic motion. Diminished active motion at high oxygen scavenger concentrations was attributed to catalytic site blocking by adsorbed solute.

publication date

  • October 8, 2024

has restriction

  • closed

Date in CU Experts

  • October 2, 2024 7:59 AM

Full Author List

  • Baghdady EA; Medlin JW; Schwartz DK

author count

  • 3

Other Profiles

Electronic International Standard Serial Number (EISSN)

  • 1520-5827

Additional Document Info

start page

  • 21097

end page

  • 21105

volume

  • 40

issue

  • 40